Why Didnt Barbara Feldon Act More?

I agree; there are quite a few movies that would have benefited from Feldon's presence (in place of the actresses actually cast).

The wikipedia article states that she's author of a published book called "Living Alone and Loving It"...which may provide a clue to the infrequency with which she accepted roles.

I quite agree. And her voice -- so melodic and soothing -- is one of the loveliest and most appealing in the history of moving image media, IMO. I could listen to her read the phone book for hours on end.

I don't think there's any denying the fact that she could have had a 'bigger' career if she'd really wanted it. Maybe she wouldn't have been 'who' she wanted to be if that had been the case, who knows? Regardless, she's a real gem in a geology set that contains lots of fool's gold (at least IMO).

She was rather typecast from her role on "Get Smart". People just couldn't stop seeing her as Agent 99.

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You have to remember the era, "tv stars" were almost never offered feature films during the 1960's and 1970's, especially after their show had ended. I guess it was snobbery more than anything because a lot of these women were quite famous and popular - Barbara Feldon, Barbara Eden, Elizabeth Montgomery, Donna Douglas, Tina Louise - I think even more so at the time than a lot of female "movie stars" who were getting the film roles. Barbara Feldon got lucky with SMILE, as very few of her tv contemporaries landed a major part in a major film at the time, usually if they did it was blatantly supporting roles (Tina Louise in THE STEPFORD WIVES) or independent movies not made by a major studio (Barbara Eden in HARPER VALLEY PTA).

She talks about it here:
http://projection-booth.blogspot.rs/2016/04/smile-bonus-interviews.html